Stretchable ionogels: Recent advances in design, toughening mechanisms, material properties and wearable devices applications

Huang, Caiyue; Jia, Xiaohua; Wang, Ding; Sun, Xisheng; Liang, Qi; Tian, Rui; Guo, Liyuan; Yang, Jin; Song, Haojie

doi:10.1016/j.cej.2024.151850

Chemical Engineering Journal

2024

DOI: 10.1016/j.cej.2024.151850

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Stretchable ionogels: Recent advances in design, toughening mechanisms, material properties and wearable devices applications

Caiyue Huang,

Xiaohua Jia,

Ding Wang

et al.

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2024

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Cited by 8 publications

References 231 publications

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Ionogels with Carbon and Organic Polymer Matrices for Electrochemical Systems

Ratajczak,

Béguin

2024

Advanced Sustainable Systems

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Ionogels (IGs) consisting of ionic liquids (ILs) confined in carbon and organic polymer matrices have recently emerged as promising materials for electrochemical systems. This perspective article explores how the structural, dynamic, and thermodynamic properties of ILs are modified by their confinement. It emphasizes the importance of combining various ILs and matrices to enhance IG properties through IL‐matrix interactions. Specifically, it highlights the significant downshift of IL melting point observed in certain porous carbons, as well as the enhanced ionic conductivity at sub‐ambient temperature in polymer networks. Accordingly, the suitability of these IGs for use in electrochemical systems operating at low temperature is discussed. Although significant progress has been made in the development and applications of carbon and polymer IGs, it is necessary to further explore the texture/structure of real host matrices, which may differ from model ones. Investigating the low‐temperature mobility of ions in IG‐based electrodes with micro/mesoporous carbons is an example of unexplored research area that may open new opportunities for increasing the energy and power density in energy storage applications. The suggested directions should facilitate innovative solutions to current and future challenges for electrochemical systems across a wide temperature range from −40 to 200 °C.

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Ionogels with Carbon and Organic Polymer Matrices for Electrochemical Systems

Ratajczak,

Béguin

2024

Advanced Sustainable Systems

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Stretchable, environmentally stable, multifunctional ionogel with self-healing and adhesive properties for high-performance flexible sensors

Wang,

Feng,

Yue

et al. 2024

Chemical Engineering Journal

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All-hydrogel yarn-based supercapacitor wrapped with multifunctional cotton fiber for energy storage and sensing

Xu,

Mao,

2024

Nano Energy

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Stretchable ionogels: Recent advances in design, toughening mechanisms, material properties and wearable devices applications

Cited by 8 publications

References 231 publications

Ionogels with Carbon and Organic Polymer Matrices for Electrochemical Systems

Ionogels with Carbon and Organic Polymer Matrices for Electrochemical Systems

Stretchable, environmentally stable, multifunctional ionogel with self-healing and adhesive properties for high-performance flexible sensors

All-hydrogel yarn-based supercapacitor wrapped with multifunctional cotton fiber for energy storage and sensing

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