2024
DOI: 10.1002/adfm.202408517
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Strong d‐p Orbital Hybridization of Os‐P via Ultrafast Microwave Plasma Assistance for Anion Exchange Membrane Electrolysis

Qichang Li,
Xiaowei Fu,
Hongdong Li
et al.

Abstract: Orbital hybridization is a promising approach to modulating the electronic structure of the designed electrocatalysts to boost reaction kinetics. In contrast to d‐d hybridization, p‐d orbital hybridization between p‐block elements and d‐block metals can provide new opportunities to modulate the electronic properties and thus promote the catalytic performance. Herein, a phosphorus‐doped osmium (P‐Os) catalyst is designed through ultrafast (20 s) microwave plasma engineering. Theoretical calculations verify the … Show more

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