To realize the applicative
potential of 2D twistronic devices,
scalable synthesis and assembly techniques need to meet stringent
requirements in terms of interface cleanness and twist-angle homogeneity.
Here, we show that small-angle twisted bilayer graphene assembled
from separated CVD-grown graphene single-crystals can ensure high-quality
transport properties, determined by a device-scale-uniform moiré
potential. Via low-temperature dual-gated magnetotransport, we demonstrate
the hallmarks of a 2.4°-twisted superlattice, including tunable
regimes of interlayer coupling, reduced Fermi velocity, large interlayer
capacitance, and density-independent Brown-Zak oscillations. The observation
of these moiré-induced electrical transport features establishes
CVD-based twisted bilayer graphene as an alternative to “tear-and-stack”
exfoliated flakes for fundamental studies, while serving as a proof-of-concept
for future large-scale assembly.