This paper focuses on the preparation and characterization of Co2FeMn full Heusler alloys using a hydrothermal route. These intermetallic compounds have a face-centered cubic crystal structure and are magnetic. The molarities used in the synthesis process were varied from 1.2 M to 2.0 M, and the resulting samples were analyzed for their structural and magnetic properties. X-ray diffraction analysis confirmed the formation of Co2FeMn Heusler alloys at molarities of 1.6 M and 1.8 M. Fourier-transform infrared spectroscopy was used to determine the transmittance in the range of 500-400 cm-1, and organic bands were observed, indicating physiochemical interactions with the environment. Vibrating sample magnetometry exhibited narrow-width M-H loops, indicating ferromagnetic behavior. The maximum magnetization was observed at a molarity of 1.8. Current-voltage (I-V) characteristics were measured for the samples with different molarities, and temperature-dependent I-V characteristics were measured for the sample prepared with a 1.8 M solution, which had a pure Co2FeMn full Heusler alloy structure.