Developing high-performance wearable electronic devices
based on
natural materials with unique structures has become a research hot
spot in the field of flexible electronics. Here, taking advantage
of natural flat silk cocoon (FSC) by controlling the spinning process
of Bombyx mori, sea urchin-like sunflower
pollen loaded with MXene nanosheets was sprayed on the FSC at a fixed
time interval to fabricate multi-layered piezoresistive sensors. The
sea urchin-like structure of SFP is beneficial to MXene loading, and
the good elasticity of sunflower pollen can withstand a large mechanical
deformation. The prepared pressure sensor has a high sensitivity of
0.028 kPa–1 and good durability, and it can respond
quickly to the applied pressure changes (response/recovery times are
140 ms/130 ms, respectively). With these excellent sensing performances,
the fabricated sensors are capable of monitoring human physiological
activities and physiological signals and can be applied in information
encryption transmission with the combination of the Morse code. The
pressure sensor developed based on the natural FSC structure shows
broad application prospects in the field of flexible wearable electronic
devices.