[13], Fe 3 O 4 /PZN-PT [14], NiFe 2 O 4 /(0 0 1) PMN-PT [15] and Ni/(1 1 0) PMN-PT [16]. Kim et al [17] studied the effects of the thickness and composition of the magnetic Co x Pd 1−x layer on the ME coupling strength. The ME constant (α) increased from 2 × 10 −7 s m −1 to 2.5 × 10 −7 s m −1 as the ilm thickness of Co 0.25 Pd 0.75 decreased from 30 nm to 10 nm. However, for both Co 0.22 Pd 0.0.78 and Co 0.18 Pd 0.0.82 compositions, α for the 10 nm thick magnetic ilm was lower than that for the 20 nm thick magnetic ilm due to the change of perpendicular magnetic anisotropy (PMA) at 10 nm. In addition, for ultrathin magnetic layers (<20 nm), the magnetostriction constant (λ) can be strongly inluenced by the thickness [18] according to the formula λ = λ b + λ i /t, where λ b is the magnetostriction of the bulk, λ i is the interfacial contribution and t is the magnetic layer thickness [19]. However, the effect of varying λ with t on ME coupling was not considered by Kim et al.
AbstractCo 50 Fe 50 /(0 1 1)-oriented lead magnesium niobate-lead titanate (PMN-PT) multiferroic (MF) heterostructures were fabricated by RF sputtering magnetic ilms onto PMN-PT substrates. The effect of magnetic layer thickness (30 nm to 100 nm) on the magnetoelectric (ME) coupling in the heterostructures was studied independently, due to the almost constant magnetostriction constant (λ = 40 ± 5 ppm) and similar as-grown magnetic anisotropies for all studied magnetic layer thicknesses. A record high remanence ratio (M r /M s ) tunability of 95% has been demonstrated in the 65 nm Co 50 Fe 50 /PMN-PT heterostructure, corresponding to a large ME constant (α) of 2.5 × 10 −6 s m −1 , when an external electric ield (E-ield) of 9 kV cm −1 was applied. Such an MF heterostructure provides considerable opportunities for E-ield-controlled multifunctional devices.