“…Nonlinear optics (NLO) is a branch of optics that describes the nonlinear relationship between dielectric polarization P and electric field E. Nonlinear optical materials have been the subject of broad research in the past few decades because of their potential applications in technological applications such as optical switching, signal processing, information storage, optical communication, laser technology, and chemical and biological species detection. [1,2] The systematic study of the NLO properties really become possible since the invention of the laser. The first nonlinear optical laser experiment was performed by Franken et al by using a ruby laser.…”