Nature-based solutions (NBSs) always provide optimal opportunities for researchers and policymakers to develop sustainable and long-term solutions for mitigating the impacts of flooding. Computing the hydrological process in hilly areas is complex compared to plain areas. This study used a laboratory-scaled hillslope model to study rainfall-runoff responses considering the natural hillslope conditions prevailing in hill torrents creating flash floods. The objective of this study was to estimate the impact of nature-based solutions on time-to-peak for flash flooding events on hilly terrains under different scenarios. Many factors decide the peak of runoff generation due to rainfall, like land use conditions, e.g., soil porosity, vegetation cover, rainfall intensity, and terrain slope. To reduce these complexities, the model was designed with thermopore sheets made of impermeable material. A hillslope model using NBS was designed to evaluate flood hydrograph attenuation to minimize the peak discharge (Qp) and increase time-to-peak (Tp) under varying rainfall, land cover, and drainage channel slope conditions. A rainfall simulator was used to analyze the formation of hydrographs for different conditions, e.g., from barren to vegetation under three different slopes (S0, S1, S2) and three rainfall intensities (P1, P2, P3). Vegetation conditions used were no vegetation, rigid vegetation, flexible vegetation, and the combination of both rigid and flexible vegetation. The purpose of using all these conditions was to determine their mitigation effects on flash flooding. This experimental analysis shows that the most suitable case to attenuate a flood hydrograph was the mixed vegetation condition, which can reduce the peak discharge by 27% to 39% under different channel slopes. The mixed vegetation condition showed an increase of 49% in time-to-peak (Tp) compared to the no vegetation condition. Additionally, under P1 rainfall and a bed slope of 0°, it reduced the peak discharge by up to 35% in the simulated flood and effectively minimized its potentially destructive impacts.