In this paper, We focused on the Lapalce eigenvalue problem which solved by Chebyshev spectral based on Lagrange polynomial. The application background of this problem is mainly light film vibration, thermal magnetic radiation, and lattice vibration, etc. This paper used spectral theory to solve the Laplace eigenvalues with high-precision. Through compared we found that our method is better than the other linear finite element method, because Chebyshev spectral method is a global approximation, it has achieved superconvergence, spectral accuracy, and easier programming, we also analysis the error of this method and projecting the eigenvectors in this paper, we found that the eigenvalue vector was approximated by this method which has more stability and smoothly. At the same time, this method also provides a new and effective reference for solving Laplace eigenvalue problem.