Sunlight induced efficient photocatalytic oxidation of benzylamines and CO<sub>2</sub> reduction over a 2D–2D MoS<sub>2</sub>/FP-BTA heterojunction catalyst

Das, Surya; Sarkar, Priyanka; Kothari, Anil Chandra; Goswami, Manoj; Khan, Aslam; Islam, Sk. Manirul

doi:10.1039/d3nj04669a

New J. Chem.

2024

DOI: 10.1039/d3nj04669a

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Sunlight induced efficient photocatalytic oxidation of benzylamines and CO₂ reduction over a 2D–2D MoS₂/FP-BTA heterojunction catalyst

Surya Das,

Priyanka Sarkar,

Anil Chandra Kothari

et al.

Abstract: The photocatalytic production of fuels and chemicals utilizing highly effective catalysts has garnered a lot of interest as a sustainable and clean strategy. Herein, we have reported the effective fabrication...

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Cited by 3 publications

References 70 publications

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Cu_xO_y Incorporated COF: A Potential Reusable Catalyst for the Synthesis of α‐Hydroxy Ketones and Oxazolidinones Under Atmospheric CO₂ Pressure and Solvent‐Free Conditions

Roy,

Sarkar,

Shahidul Islam

et al. 2024

ChemCatChem

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In this present work, a newly designed metal nanoparticle associated Covalent organic framework (COF), CuxOy@TFP‐ODA has been successfully synthesized and used for the effective synthesis of Oxazolidinones and a‐hydroxy ketones under mild conditions utilizing CO2. Initially, imine‐linked 2D COF, TFP‐ODA was synthesized by simple solvothermal method followed by the embedment of copper nanoparticles (NPs) into the skeleton of the as‐synthesized COF. Different characterization techniques were employed to establish the physical and chemical characteristics of both CuxOy@TFP‐ODA and TFP‐ODA COF materials. To study the catalytic efficiency of the highly porous CuxOy@TFP‐ODA, three components coupling reaction involving primary amine, propargyl alcohol and CO2 to synthesize a series of 2‐Oxazolidinone and synthesis of α‐hydroxy ketones using CO2 as a Co‐catalyst were carried out over the as‐prepared catalyst under green and sustainable conditions which illustrated excellent yields and selectivity of the corresponding products. The synthesized catalyst was proved to be completely heterogeneous and especially, the catalyst material demonstrated significant potential for reuse across several catalytic cycles.

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Cu_xO_y Incorporated COF: A Potential Reusable Catalyst for the Synthesis of α‐Hydroxy Ketones and Oxazolidinones Under Atmospheric CO₂ Pressure and Solvent‐Free Conditions

Roy,

Sarkar,

Shahidul Islam

et al. 2024

ChemCatChem

View full text Add to dashboard Cite

show abstract

Solar-driven triple photocatalytic action of defective S-doped g-C₃N₄ for 1,4 NADH regeneration and simultaneous benzylamine conversion along with CO₂ fixation into HCOOH

Sharma,

Yadav,

Verma

et al. 2024

Catal. Sci. Technol.

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Utility of silver nanoparticles embedded on a covalent organic framework as a highly active catalyst for carboxylative cyclization with CO₂: a sustainable route for production of tetronic acids and oxazolidinones

Nandi,

Haque,

Biswas

et al. 2024

New J. Chem.

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Sunlight induced efficient photocatalytic oxidation of benzylamines and CO₂ reduction over a 2D–2D MoS₂/FP-BTA heterojunction catalyst

Abstract: The photocatalytic production of fuels and chemicals utilizing highly effective catalysts has garnered a lot of interest as a sustainable and clean strategy. Herein, we have reported the effective fabrication...

Cited by 3 publications

References 70 publications

Cu_xO_y Incorporated COF: A Potential Reusable Catalyst for the Synthesis of α‐Hydroxy Ketones and Oxazolidinones Under Atmospheric CO₂ Pressure and Solvent‐Free Conditions

Cu_xO_y Incorporated COF: A Potential Reusable Catalyst for the Synthesis of α‐Hydroxy Ketones and Oxazolidinones Under Atmospheric CO₂ Pressure and Solvent‐Free Conditions

Solar-driven triple photocatalytic action of defective S-doped g-C₃N₄ for 1,4 NADH regeneration and simultaneous benzylamine conversion along with CO₂ fixation into HCOOH

Utility of silver nanoparticles embedded on a covalent organic framework as a highly active catalyst for carboxylative cyclization with CO₂: a sustainable route for production of tetronic acids and oxazolidinones

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Sunlight induced efficient photocatalytic oxidation of benzylamines and CO2 reduction over a 2D–2D MoS2/FP-BTA heterojunction catalyst

Abstract: The photocatalytic production of fuels and chemicals utilizing highly effective catalysts has garnered a lot of interest as a sustainable and clean strategy. Herein, we have reported the effective fabrication...

Cited by 3 publications

References 70 publications

CuxOy Incorporated COF: A Potential Reusable Catalyst for the Synthesis of α‐Hydroxy Ketones and Oxazolidinones Under Atmospheric CO2 Pressure and Solvent‐Free Conditions

CuxOy Incorporated COF: A Potential Reusable Catalyst for the Synthesis of α‐Hydroxy Ketones and Oxazolidinones Under Atmospheric CO2 Pressure and Solvent‐Free Conditions

Solar-driven triple photocatalytic action of defective S-doped g-C3N4 for 1,4 NADH regeneration and simultaneous benzylamine conversion along with CO2 fixation into HCOOH

Utility of silver nanoparticles embedded on a covalent organic framework as a highly active catalyst for carboxylative cyclization with CO2: a sustainable route for production of tetronic acids and oxazolidinones

Contact Info

Product

Resources

About

Sunlight induced efficient photocatalytic oxidation of benzylamines and CO₂ reduction over a 2D–2D MoS₂/FP-BTA heterojunction catalyst

Cu_xO_y Incorporated COF: A Potential Reusable Catalyst for the Synthesis of α‐Hydroxy Ketones and Oxazolidinones Under Atmospheric CO₂ Pressure and Solvent‐Free Conditions

Cu_xO_y Incorporated COF: A Potential Reusable Catalyst for the Synthesis of α‐Hydroxy Ketones and Oxazolidinones Under Atmospheric CO₂ Pressure and Solvent‐Free Conditions

Solar-driven triple photocatalytic action of defective S-doped g-C₃N₄ for 1,4 NADH regeneration and simultaneous benzylamine conversion along with CO₂ fixation into HCOOH

Utility of silver nanoparticles embedded on a covalent organic framework as a highly active catalyst for carboxylative cyclization with CO₂: a sustainable route for production of tetronic acids and oxazolidinones