Superconducting MoC thin films with enhanced sheet resistance

We investigate the complex conductivity of a highly disordered MoC superconducting film with kF l ≈ 1, where kF is the Fermi wavenumber and l is the mean free path, derived from experimental transmission characteristics of coplanar waveguide resonators in a wide temperature range below the superconducting transition temperature Tc. We find that the original Mattis-Bardeen model with a finite quasiparticle lifetime, τ , offers a perfect description of the experimentally observed complex conductivity. We show that τ is appreciably reduced by scattering effects. Characteristics of the scattering centers are independently found by the scanning tunneling spectroscopy and agree with those determined from the complex conductivity.

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“…The preparation details are given in Ref. 16. The transport properties of the MoC thin films have been obtained by four-probe measurements.…”

Section: Moc Thin Film and Cpw Resonatormentioning

confidence: 99%

Finite quasiparticle lifetime in disordered superconductors

et al. 2015

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“…The details can be found elsewhere [17]. The preparation followed the procedure of Lee and Ketterson [18] who manufactured continuous MoC films down to 0.4 nm thickness showing…”

Section: Introductionmentioning

confidence: 99%

“…The details can be found elsewhere [17]. The preparation followed the procedure of Lee and Ketterson [18] The inset of Fig.…”

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Fermionic scenario for the destruction of superconductivity in ultrathin MoC films evidenced by STM measurements

et al. 2016

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We use sub-Kelvin scanning tunneling spectroscopy to investigate the suppression of superconductivity in homogeneously disordered ultrathin MoC films. We observe that the superconducting state remains spatially homogeneous even on the films of 3 nm thickness. The vortex imaging suggests the global phase coherence in our films. Upon decreasing thickness, when the superconducting transition drops from 8.5 to 1.2 K, the superconducting energy gap  follows perfectly T c . All this is pointing to a two-stage fermionic scenario of the superconductor-insulator transition (SIT) via a metallic state as an alternative to the direct bosonic SIT scenario with a Cooper-pair insulating state evidenced by the last decade STM experiments. [7][8][9][10][11][12][13] bring evidences that upon increasing disorder decreases more slowly than T c , the variation of on a scale of the superconducting coherence length  increases, a pseudogap appears above T c in the tunneling spectra, the spectral coherence peaks are suppressed, and the vortex lattice is fading out. This phenomenology strongly supports the bosonic scenario and raises the question about the universality of the bosonic SIT [14]. On the other hand, potential evidence for the fermionic mechanism was provided even sooner by the tunneling experiments on planar junctions on amorphous Bi and PbBi/Ge films [15,16] indicating that the Cooper pair amplitude vanishes at SIT. But the unambiguousness of these results was challenged by the fact that the spatially averaged tunneling spectra were gapless. This gaplessness could be explained by a very inhomogeneous gap distribution due to phase fluctuations. Then, superconducting pair correlations might also exist in insulators close to SIT, contradicting the fermionic scenario. KeywordsHere, we present sub-Kelvin STM experiments on ultra thin superconducting MoC films with atomic spatial resolution. We demonstrate the spatial homogeneity of the superconducting state for film thicknesses down to 3 nm and the closing of the superconducting energy gap/order parameter as T c vanishes, in agreement with the fermionic scenario. Thus, we bring the first direct evidence on the local behavior of the superconducting order parameter in this class of the transition.The MoC films were prepared by the magnetron reactive sputtering from a Mo target in an argon-acetylene atmosphere onto a sapphire c-cut substrate. The details can be found elsewhere [17]. The preparation followed the procedure of Lee and Ketterson [18] who manufactured continuous MoC films down to 0.4 nm thickness showing

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“…MoC films of 3 nm thickness were prepared by the reactive magnetron sputtering onto a Si substrate as described in [12,13]. The Ioffe-Regel parameter kFl was determined for all our thin MoC films [6,12] from the free-electron-model. Transport and STM measurements were performed in magnetic fields up to 16 and 8 T, respectively, all at temperatures down to 0.3 K. Details are in Suppl.…”

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Zeeman-driven superconductor-insulator transition in strongly disordered MoC films: Scanning tunneling microscopy and transport studies in a transverse magnetic field

et al. 2020

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Superconductor insulator transition in transverse magnetic field is studied in the highly disordered MoC film with the product of the Fermi momentum and the mean free path kF*l close to unity. Surprisingly, the Zeeman paramagnetic effects dominate over orbital coupling on both sides of the transition. In superconducting state it is evidenced by a high upper critical magnetic field 2 , by its square root dependence on temperature, as well as by the Zeeman splitting of the quasiparticle density of states (DOS) measured by scanning tunneling microscopy. At 2 a logarithmic anomaly in DOS is observed. This anomaly is further enhanced in increasing magnetic field, which is explained by the Zeeman splitting of the Altshuler-Aronov DOS driving the system into a more insulating or resistive state. Spin dependent Altshuler-Aronov correction is also needed to explain the transport behavior above 2 .

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Superconducting MoC thin films with enhanced sheet resistance

Cited by 10 publications

References 6 publications

Finite quasiparticle lifetime in disordered superconductors

Finite quasiparticle lifetime in disordered superconductors

Fermionic scenario for the destruction of superconductivity in ultrathin MoC films evidenced by STM measurements

Zeeman-driven superconductor-insulator transition in strongly disordered MoC films: Scanning tunneling microscopy and transport studies in a transverse magnetic field

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