Over the past two decades, several molecules have been explored as possible building blocks of a quantum computer, a device that would provide exponential speedups for a number of problems, including the simulation of large, strongly correlated chemical systems. Achieving strong interactions and entanglement between molecular qubits remains an outstanding challenge. Here, we show that the TbPc 2 single-molecule magnet has the potential to overcome this obstacle due to its sensitivity to electric fields stemming from the hyperfine Stark effect. We show how this feature can be leveraged to achieve long-range entanglement between pairs of molecules using a superconducting resonator as a mediator. Our results suggest that the molecule-resonator interaction is near the edge of the strong-coupling regime and could potentially pass into it given a more detailed, quantitative understanding of the TbPc 2 molecule.
Graphical TOC EntryKeywords single molecule magnet, TbPc 2 molecule, long-range entanglement, hyperfine Stark effect, superconducting resonator, strong-coupling limit Recently, a qubit candidate with remarkable properties was experimentally demonstrated by Thiele et al.: 16 the SMM TbPc 2 , which features a nuclear spin as the qubit, with the attractive and unusual property of being electrically controllable. This combines the best of both worlds: long-lived qubit coherence with fast controllability. This recent exciting