directional coupling between propagating photons and surface plasmon polaritons (SPPs) in the visible range is a growing pursuit, due to its perceived essential role in nanoplasmonic and nanophotonic applications. [11][12][13] Here, we demonstrate that asymmetric, two-element, periodic, metal-insulator-metal (MIM) structures, perhaps representing the simplest gradient-index scenario, can serve as refl ectionless directional converters between free photons and SPPs operable in the visible frequency range. The simplicity of this two-element MIM structure allows for the fabrication of testable samples for operation with visible light. Simulated dispersion relations of this structure reveal the nature of the high-effi ciency coupling process: interactions between propagating modes caused by the broken refl ection symmetry (RS) and localized modes generated by individual MIM elements that are well understood in the language of MM "perfect absorbers". [ 14,15 ] There are regions in k -space where these interactions are very strong, such that the two modes hybridize to two new quasi-particles, [ 16,17 ] with concomitant Rabi splitting. [ 18,19 ] Experiments on samples with tuned parameters confi rm the simulated dispersion maps, and demonstrate a large Rabi splitting. Absolute refl ectance measurements under normal incidence with small aperture angle (3.75°) on samples with areas less than 60 × 60 µm 2 were carried out using a modifi ed microscope design. This scheme avoids the common problem of averaging over large incident angles when measuring optical properties of small-area samples by conventional methods. [ 20 ] Direct experimental evidence is obtained for refl ectionless (less than 8% measured refl ectance) directional SPP coupling in the visible range, with more than 88.8% of the channeled SPP energy being directed to the designed direction. Our results are meaningful for integrated nanoplasmonics, plasmonic logic, and plasmonic light harvesting, among others.
Results and Discussions
Localized Mode AnalysisUsing the measurement scheme described in Experimental Section, we performed refl ectance measurements to study Gradient-index meta-surfaces have been shown to have the ability to manipulate wavefronts at will in a refl ectionless manner in the GHz range, including the extreme example of converting freely propagating waves into surface waves with high effi ciency. Upon approaching the optical regime, the gradient-index concept encounters diffi culties due to fabrication limitations. Here, it is theoretically and experimentally demonstrated that asymmetric, periodic, two-element metal-insulator-metal structures can serve as refl ectionless directional converters between freely propagating visible photons and surface plasmon polaritons (SPPs). Coupling between propagating modes caused by the broken symmetry and localized modes generated by individual elements is shown to be the mechanism of this high-effi ciency process, yielding an observed Rabi splitting of ∼135 meV. Direct experimental evidence is obtained fo...