2023
DOI: 10.1002/ange.202305719
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Supramolecular Enhancement of Electrochemical Nitrate Reduction Catalyzed by Cobalt Porphyrin Organic Cages for Ammonia Electrosynthesis in Water**

Abstract: The electrochemical nitrate (NO3−) reduction reaction (NO3RR) to ammonia (NH3) represents a sustainable approach for denitrification to balance global nitrogen cycles and an alternative to traditional thermal Haber‐Bosch processes. Here, we present a supramolecular strategy for promoting NH3 production in water from NO3RR by integrating two‐dimensional (2D) molecular cobalt porphyrin (CoTPP) units into a three‐dimensional (3D) porous organic cage architecture. The porphyrin box CoPB‐C8 enhances electrochemical… Show more

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Cited by 3 publications
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