The high-current pulsed electron beam (HCPEB) treatment with current density 6 J/cm 2 was applied on AZ91 Mg alloy to improve its corrosion resistance. Results showed that the net-like Mg 17 Al 12 disappeared on the surface of AZ91 Mg alloy after irradiation by HCPEB, which was instead of supersaturated Al element on the surface. Nevertheless, the application of HCPEB also led to the formation of crater-like and groove-like structures as well as micro-cracks on the surface of AZ91 Mg alloy. After HCPEB treatment by 3, 5 and 10 pulses, the AZ91 Mg alloy exhibited better corrosion resistance. However, the increasing amount of micro-cracks reduced the anti-corrosive properties of AZ91 Mg alloy as the pulse increased to 20 and 30. Keywords High-current pulsed electron beam (HCPEB) Á Corrosion resistance Á Electrochemical impedance spectroscopy (EIS) Á AZ91 Mg alloy Á Microstructure