2022
DOI: 10.1021/acssuschemeng.2c03397
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Surface/Lattice Oxygen Synergism of Durable CuO Catalysts for Tandem Dehydrogenation–Oxidation of Glycerol to Carboxylic Acids in Oxygen-Free Medium

Abstract: Catalytic dehydrogenation–oxidation of bio-oxygenates to carboxylic acids and green H2 has been considered a key technology for biorefineries. Composition, size, and morphology are critical parameters for solid catalysts. However, the synergism of surface/lattice oxygen in inexpensive metal oxide catalysts is largely unexplored in this area. In this work, a systematic study on the surface/lattice oxygen synergism of crystallized CuO catalysts has been performed using glycerol dehydrogenation as an example. The… Show more

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