2014
DOI: 10.1039/c4ra05787b
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Surface passivation assisted lasing emission in the quantum dots doped cholesteric liquid crystal resonating cavity with polymer template

Abstract: A copolymer has been used as a template for enhanced optical properties of core–shell CdS/ZnSe quantum dots doped cholesteric liquid crystal.

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Cited by 13 publications
(11 citation statements)
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“…Thus, CLCs are usually considered a 1D photonic crystal with an adjustable photonic bandgap (PBGs) via the temperature dependence of the pitch P. After doping the gain medium (e.g., dyes and QDs), the CLC helix acts as a resonator necessary for laser emission, which can be tuned by various external stimuli. Compared to conventional LC lasers, which are fabricated by dispersing laser dyes into CLCs, LC lasers based on QDs can lase emissions with improved features such as narrower line width, lower lasing threshold and low intensity to noise ratios, as well as high stability due to the 3D quantum confinement effect of QDs [131,[299][300][301] (Figure 11). On the other hand, amplified spontaneous emission (ASE) from colloids of QDs dispersed in LCs has also been investigated widely [301].…”
Section: Photonic Applicationsmentioning
confidence: 99%
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“…Thus, CLCs are usually considered a 1D photonic crystal with an adjustable photonic bandgap (PBGs) via the temperature dependence of the pitch P. After doping the gain medium (e.g., dyes and QDs), the CLC helix acts as a resonator necessary for laser emission, which can be tuned by various external stimuli. Compared to conventional LC lasers, which are fabricated by dispersing laser dyes into CLCs, LC lasers based on QDs can lase emissions with improved features such as narrower line width, lower lasing threshold and low intensity to noise ratios, as well as high stability due to the 3D quantum confinement effect of QDs [131,[299][300][301] (Figure 11). On the other hand, amplified spontaneous emission (ASE) from colloids of QDs dispersed in LCs has also been investigated widely [301].…”
Section: Photonic Applicationsmentioning
confidence: 99%
“…The optical excitation and emission of these nanomaterials could be tuned effectively through the interaction between nanomaterials and the long-range ordered LC molecules, leading to a series of potential applications such as information storage, displays, LC lasers, etc. [130][131][132][133][134].…”
Section: Introductionmentioning
confidence: 99%
“…As an alternative to conventional organic dyes, some inorganic quantum dots (QDs) with relatively narrow emission bands and high brightness have been introduced to obtain wavelengthtunable CPL, thus avoiding emission quenching. [35][36][37][38][39][40][41] Despite these advantages, the main problem of embedding QDs into the LC medium is that it is hard to attain a high concentration of QDs while retaining the optical properties. Another problem is that QDs tend to aggregate inside the LCs.…”
Section: Communicationmentioning
confidence: 99%
“…We estimated the pitch as p = 0.43 lm by using the relation above and considering HTP = +6.67 lm À1 for the chiral dopant CB15. When the Ch-sample was sandwiched between two glass-slides as described above the planar texture (or Grandjen) was observed under POM at 24.1°C, this texture is quite stable [6][7][8][9] and we observed that the optical properties are still stable over more than one year. In Fig.…”
Section: Ch-lc Samplementioning
confidence: 76%
“…On the other hand, when the temperature increases, the springs are compressed and the reflected wavelengths are shorter (hypsochromic shift) [4,5]. Furthermore, these materials feature sufficient optical stability for many applications [6][7][8][9]. The main applications of chiral macrostructures include: bistable cholesteric reflective displays [10][11][12][13][14], optical filter for circularly polarized light in LCDs [15], electrically switchable mirrors [16], chiral pharmaceutical resolution [17], and photonic band gap materials [18,19].…”
Section: Introductionmentioning
confidence: 99%