Surface Plasmon Enhanced Strong Exciton–Photon Coupling in Hybrid Inorganic–Organic Perovskite Nanowires

Abstract

Manipulating strong light-matter interaction in semiconductor microcavities is crucial for developing high-performance exciton polariton devices with great potential in next-generation all-solid state quantum technologies. In this work, we report surface plasmon enhanced strong exciton-photon interaction in CHNHPbBr perovskite nanowires. Characteristic anticrossing behaviors, indicating a Rabi splitting energy up to ∼564 meV, are observed near exciton resonance in hybrid perovskite nanowire/SiO/Ag cavity at room temperature. The exciton-photon coupling strength is enhanced by ∼35% on average, which is mainly attributed to surface plasmon induced localized excitation field redistribution. Further, systematic studies on SiO thickness and nanowire dimension dependence of exciton-photon interaction are presented. These results provide new avenues to achieve extremely high coupling strengths and push forward the development of electrically pumped and ultralow threshold small lasers.

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“…g) Electric field distributions in the NW on the glass (left) and 5 nm SiO 2 /Ag (right) substrates. (a)–(g) Reproduced with permission . Copyright 2018, American Chemical Society.…”