Synergy effect of highly dispersed palladium and Ni-SiW polyoxometalate-based metal-organic framework (POMOF) for highly efficient and selective nitroaromatics hydrogenation

Liu, Qingqing; Zhong, Yi; Fu, Huan; Wang, Qianqian; Zhu, Lihua

doi:10.1016/j.apcata.2023.119373

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2024

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Cited by 3 publications

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“…142 Consequently, collaborative interactions with other enzyme-mimicking substances are anticipated to advance the detection of biologically active compounds significantly. 143…”

Section: Challenges and Prospectsmentioning

confidence: 99%

Advancing biomedical applications of polyoxometalate-based metal–organic frameworks: from design to therapeutic potential

Wang,

Dai,

et al. 2024

Inorg. Chem. Front.

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“…142 Consequently, collaborative interactions with other enzyme-mimicking substances are anticipated to advance the detection of biologically active compounds significantly. 143…”

Section: Challenges and Prospectsmentioning

confidence: 99%

Advancing biomedical applications of polyoxometalate-based metal–organic frameworks: from design to therapeutic potential

Wang,

Dai,

et al. 2024

Inorg. Chem. Front.

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Highly Dispersed Palladium Nanoparticles on Carbon Doping with Nitrogen Derived from MOFs for 4‐Nitrophenol Hydrogenation

Wang,

Yuan,

Zhang

et al. 2024

ChemistrySelect

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A series of the Pd/NC samples with various Pd loadings (0.11%, 0.48%, and 2.52%) are prepared via sodium borohydride (NaBH4) reduction method and carbon doping with nitrogen (NC) is acquired by the pyrolysis of ZIF‐8. The samples are characterized by XRD, BET, SEM, TEM, HRTEM, STEM‐EDX elemental maps and line‐scanning, XPS, TG, and so forth. It confirms that the Pd nanoparticles (NPs) are successfully coated on the NC. The catalytic behaviors of the samples are evaluated by the hydrogenation of 4‐nitrophenol (4‐NP), the 2.52%Pd/NC catalyst shows the best catalytic property among as‐obtained catalysts maybe due to the much more Pd(0) species. The 2.52%Pd/NC catalyst exhibits 100% selectivity to 4‐aminophenol (4‐AP) at high conversion of 4‐nitrophenol and 321.8 h−1 turnover frequency (TOF) under mild reaction conditions (3.0 MPa H2, 40 °C, 1 h). Moreover, the catalysts show an excellent stability.

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Highly dispersed Pd nanoparticles supported by magnetically separable Fe3O4@ SiO2 nanotube for catalytic hydrogenation of nitroaromatics

Sheng,

Xia,

2024

Journal of Colloid and Interface Science

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Synergy effect of highly dispersed palladium and Ni-SiW polyoxometalate-based metal-organic framework (POMOF) for highly efficient and selective nitroaromatics hydrogenation

Cited by 3 publications

References 44 publications

Advancing biomedical applications of polyoxometalate-based metal–organic frameworks: from design to therapeutic potential

Advancing biomedical applications of polyoxometalate-based metal–organic frameworks: from design to therapeutic potential

Highly Dispersed Palladium Nanoparticles on Carbon Doping with Nitrogen Derived from MOFs for 4‐Nitrophenol Hydrogenation

Highly dispersed Pd nanoparticles supported by magnetically separable Fe3O4@ SiO2 nanotube for catalytic hydrogenation of nitroaromatics

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