Synthesis and investigation of a <i>meta</i>[6]cycloparaphenylene gold(<scp>i</scp>) <i>N</i>-heterocyclic carbene complex

Bernt, Felix; Leonhardt, Christopher M.; Schatz, Dominic; Wegner, Hermann A.

doi:10.1039/d3cc06225b

Chem. Commun.

2024

DOI: 10.1039/d3cc06225b

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Synthesis and investigation of a meta[6]cycloparaphenylene gold(i) N-heterocyclic carbene complex

Felix Bernt,

Christopher M. Leonhardt,

Dominic Schatz

et al.

Abstract: Meta[n]cycloparaphenylenes (m[n]CPPs) as well as N-heterocyclic carbene (NHC) gold(I)-complexes are intriguing building blocks for material and life sciences due to their extraordinary structures resulting in unique photophysical properties. Herein, we...

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Cited by 3 publications

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Synthesis of All‐Benzene Multi‐Macrocyclic Nanocarbons by Post‐Functionalization of meta‐Cycloparaphenylenes

Gao,

Bu,

Chen

et al. 2024

Angewandte Chemie

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Expanding the diversity of multi‐macrocyclic nanocarbons, particularly those with all‐benzene scaffolds, represents intriguing yet challenging synthetic tasks. Complementary to the existing synthetic approaches, here we report an efficient and modular post‐functionalization strategy employing iridium‐catalyzed C–H borylation of the highly strained meta‐cycloparaphenylenes (mCPPs) and an mCPP‐derived catenane. Based on the functionalized macrocyclic synthons, a number of novel all‐benzene topological structures including linear and cyclic chains, polycatenane, and pretzelane have been successfully prepared and characterized, thereby showcasing the synthetic utility and potential of the post‐functionalization strategy.

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Synthesis of All‐Benzene Multi‐Macrocyclic Nanocarbons by Post‐Functionalization of meta‐Cycloparaphenylenes

Gao,

Bu,

Chen

et al. 2024

Angewandte Chemie

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Synthesis of All‐Benzene Multi‐Macrocyclic Nanocarbons by Post‐Functionalization of meta‐Cycloparaphenylenes

Gao,

Bu,

Chen

et al. 2024

Angew Chem Int Ed

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Viologen–cycloparaphenylene hybrids: luminescent molecular nanocarbons for anion binding and specific vapor sorption

Frydrych,

Senthilkumar,

Ślusarek

et al. 2025

Org. Chem. Front.

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Synthesis and investigation of a meta[6]cycloparaphenylene gold(i) N-heterocyclic carbene complex

Abstract: Meta[n]cycloparaphenylenes (m[n]CPPs) as well as N-heterocyclic carbene (NHC) gold(I)-complexes are intriguing building blocks for material and life sciences due to their extraordinary structures resulting in unique photophysical properties. Herein, we...

Cited by 3 publications

References 28 publications

Synthesis of All‐Benzene Multi‐Macrocyclic Nanocarbons by Post‐Functionalization of meta‐Cycloparaphenylenes

Synthesis of All‐Benzene Multi‐Macrocyclic Nanocarbons by Post‐Functionalization of meta‐Cycloparaphenylenes

Synthesis of All‐Benzene Multi‐Macrocyclic Nanocarbons by Post‐Functionalization of meta‐Cycloparaphenylenes

Viologen–cycloparaphenylene hybrids: luminescent molecular nanocarbons for anion binding and specific vapor sorption

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