2024
DOI: 10.3390/ma17081712
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Synthesis and Transport Properties of ZnSnP2-yAsy Chalcopyrite Solid Solutions

Daniel Ramirez,
Luke T. Menezes,
Holger Kleinke

Abstract: This work focuses on the synthesis and properties of quaternary ZnSnP2-yAsy chalcopyrite solid solutions. Full miscibility of the solid solution is achieved using ball milling followed by hot press sintering. The measured electrical conductivity increases substantially with As substitution from 0.03 S cm−1 for ZnSnP2 to 10.3 S cm−1 for ZnSnAs2 at 715 K. Band gaps calculated from the activation energies show a steady decrease with increasing As concentration from 1.4 eV for ZnSnP2 to 0.7 eV for ZnSnAs2. The See… Show more

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