2024
DOI: 10.1002/cctc.202401279
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Synthesis, Structure, and Catalytic Reactivity of Bioinspired Models of Calcium‐ and Lanthanide‐Dependent Methanol Dehydrogenase

Mianran Chao,
Chaoyue Sun,
Xuan Zhang
et al.

Abstract: It has been a long‐standing goal for chemists to develop selective catalytic oxidation systems with molecular oxygen as a green terminal oxidant from the inspiration of active sites in natural metalloenzymes. Lanthanide‐centered methanol dehydrogenase (Ln‐MDH), which contained the same pyrroloquinoline quinone (PQQ) redox cofactor as the analogous calcium‐based MDH (Ca‐MDH) and exhibited good reactivity in alcohol oxidation, was discovered in 2011 and had aroused extensive research interest during the past dec… Show more

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