A single
photodetector with tunable detection wavelengths and polarization
sensitivity can potentially be harnessed for diverse optical applications
ranging from imaging and sensing to telecommunications. Such a device
will require the combination of multiple material systems with different
structures, band gaps, and photoelectrical responses, which is extremely
difficult to engineer using traditional epitaxial films. Here, we
develop a multifunctional and high-performance photosensor using all
van der Waals materials. The device features a gate-tunable spectral
response that is switchable between near-infrared/visible and short-/midwave
infrared, as well as broad-band operation, at room temperature. The
linear polarization sensitivity in the telecommunication O-band can
also be directly modulated between horizontal, vertical, and nonpolarizing
modes. These effects originate from the balance of photocurrent generation
in two of the active layers that can be manipulated by an electric
field. The photodetector features high detectivity (>109 cmHz1/2W–1) together with fast operation
speed (∼1 MHz) and can be further exploited for dual visible
and infrared imaging.