2024
DOI: 10.1002/ange.202408937
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Taming Two‐Dimensional Polymerization by a Machine‐Learning Discovered Crystallization Model

Jiaxin Tian,
Kiana A. Treaster,
Liangtao Xiong
et al.

Abstract: Rapidly synthesizing high‐quality two‐dimensional covalent organic frameworks (2D COFs) is crucial to their practical applications. Here, we use a machine‐learning approach that overcomes the challenges associated with bottom‐up model derivation for the non‐classical 2D COF crystallization processes. The resulting model, referred to as NEgen1, establishes correlations among the induction time, nucleation rate, growth rate, bond‐forming rate constants, and common solution synthesis conditions for 2D COFs that g… Show more

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