2022
DOI: 10.1016/j.ijbiomac.2022.04.099
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Tannic acid modified antifreezing gelatin organohydrogel for low modulus, high toughness, and sensitive flexible strain sensor

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Cited by 34 publications
(24 citation statements)
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“…In addition to the mechanical reinforcement, TA is able to improve the flexibility and energy dissipation of hydrogel due to the formation of non-covalent interactions, which can easily recover the broken bonds after the deformation. 267 TA concentration is the determining factor for mechanical properties improvement. Although a critical concentration of TA and polymers is needed for the hydrogelation, a further increase of TA/polymers concentration from a certain point can lead to a decrease in mechanical properties due to the inhomogeneity of hydrogels coagulation during the mixing and fast gelation.…”
Section: Ta-based Hydrogelsmentioning
confidence: 99%
“…In addition to the mechanical reinforcement, TA is able to improve the flexibility and energy dissipation of hydrogel due to the formation of non-covalent interactions, which can easily recover the broken bonds after the deformation. 267 TA concentration is the determining factor for mechanical properties improvement. Although a critical concentration of TA and polymers is needed for the hydrogelation, a further increase of TA/polymers concentration from a certain point can lead to a decrease in mechanical properties due to the inhomogeneity of hydrogels coagulation during the mixing and fast gelation.…”
Section: Ta-based Hydrogelsmentioning
confidence: 99%
“…44,45 Although natural polymers such as gelatin lack self-healing properties, [46][47][48][49][50] introducing TA facilitates excellent multifunctionality, including tunable mechanical strength and self-healing, in gelatin hydrogels. [51][52][53] Similarly, although alginate and chitosan (CS) are excellent natural polymers for hydrogel formation, they lack self-healing and adhesive capabilities in their native form. Inducing selfhealing and adhesive properties requires laborious and timeconsuming procedures, [20][21][22] which can impede the practical adoption of hydrogels for fabricating strain sensors.…”
Section: Multifunctionality Of Small Biomolecules In Hydrogel-based S...mentioning
confidence: 99%
“…16(b)). 51 Phytic acid (PA) PA contains a high phosphorus and carbon content, making it a biogenic and non-toxic compound. PA is naturally derived from oilseeds, legumes, cereals, nuts, fruits, vegetables, pollen, seeds, roots, and plant stems.…”
Section: Zwitterionic Osmolytesmentioning
confidence: 99%
“…14−16 This is because most naturally derived biomolecules exhibit excellent biodegradability and recyclability. 17 molecule in many papers on sensor systems. 18−20 Our group recently reported that ATP can behave as an "all-in-one" green FR because it contains three major components that can lead to intumescent char formation: three PO 4 3− groups that serve as an acid source, a five-carbon monosaccharide ribose sugar that promotes char formation, and a nucleobase with amine groups that act as a blowing agent.…”
Section: Introductionmentioning
confidence: 99%
“…Several biomolecules, such as deoxyribonucleic acid (DNA), proteins, and lignin, are of great interest as green FRs. This is because most naturally derived biomolecules exhibit excellent biodegradability and recyclability . Adenosine triphosphate (ATP) is a well-known abundant biomolecule involved in energy transport and has appeared as a target molecule in many papers on sensor systems. Our group recently reported that ATP can behave as an “all-in-one” green FR because it contains three major components that can lead to intumescent char formation: three PO 4 3– groups that serve as an acid source, a five-carbon monosaccharide ribose sugar that promotes char formation, and a nucleobase with amine groups that act as a blowing agent .…”
Section: Introductionmentioning
confidence: 99%