Nanosilica was synthesized via the hydrothermal technique, followed by the vacuum frying system at low temperature and pressure. Then, the achieved nanoparticles were used for removing of Crystal Violet dye (CV) from wastewater. The absorbent and absorption process were studied by Fourier transform infrared spectroscopy (FTIR), X-ray diffraction (XRD), Field Emission Scanning Electron Microscope (FE-SEM), X-ray Fluorescence (XRF). Batch adsorption experiments were conducted under different conditions including contact time, initial concentration of dye and adsorbent dose. The kinetic study of CV dye on the nanoparticles can be well depicted theoretically by using pseudo-second-order kinetic model.