The crucial role of hydrogen bonding in shaping the structures of zinc-based coordination polymers using tridentate N, N, O donor reduced Schiff base ligands and bridging acetates

Middya, Puspendu; Frontera, Antonio; Chattopadhyay, Shouvik

doi:10.1039/d4ra00550c

RSC Adv.

2024

DOI: 10.1039/d4ra00550c

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The crucial role of hydrogen bonding in shaping the structures of zinc-based coordination polymers using tridentate N, N, O donor reduced Schiff base ligands and bridging acetates

Puspendu Middya,

Antonio Frontera,

Shouvik Chattopadhyay

Abstract: In this article synthesis, characterization and DFT study of two polynuclear zinc(ii) complexes with reduced Schiff base have been reported.

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Synthesis, Structural Characterization, and Theoretical Analysis of Nonconventional Bonding in Dinuclear Zinc(II) Complexes with Tridentate Schiff Bases

Halder,

Middya,

Gomila

et al. 2024

ACS Omega

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Two tridentate N,N,O-donor ligands, HL 1 = 4-chloro-2-(((2-(methylamino)ethyl)amino)methyl)phenol and HL 2 = 4-chloro-2-(((2-(dimethylamino)ethyl)amino)methyl)phenol, have been used to synthesize phenolate-bridged dinuclear complexes [Zn 2 (L 1 ) 2 Cl 2 ] ( 1) and [Zn 2 (L 2 ) 2 (N 3 ) 2 ] (2). Single-crystal X-ray diffraction analysis confirmed their structures. Both complexes form assemblies in the solid state. Moreover, the existence of nonconventional spodium bonds in 1 and tetrel bonds in 2 has been explored using theoretical calculations, including MEP surface plots and QTAIM and NCIplot analyses.

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Synthesis, Structural Characterization, and Theoretical Analysis of Nonconventional Bonding in Dinuclear Zinc(II) Complexes with Tridentate Schiff Bases

Halder,

Middya,

Gomila

et al. 2024

ACS Omega

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show abstract

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The crucial role of hydrogen bonding in shaping the structures of zinc-based coordination polymers using tridentate N, N, O donor reduced Schiff base ligands and bridging acetates

Abstract: In this article synthesis, characterization and DFT study of two polynuclear zinc(ii) complexes with reduced Schiff base have been reported.

Cited by 1 publication

References 105 publications

Synthesis, Structural Characterization, and Theoretical Analysis of Nonconventional Bonding in Dinuclear Zinc(II) Complexes with Tridentate Schiff Bases

Synthesis, Structural Characterization, and Theoretical Analysis of Nonconventional Bonding in Dinuclear Zinc(II) Complexes with Tridentate Schiff Bases

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