The divergence-free and gamma-traceless vector-spinor eigenfunctions, as well as the divergence-free and gamma-traceless rank-2 symmetric tensor-spinor eigenfunctions, of the Dirac operator on the N -sphere (S N ) are written down explicitly for N ≥ 3. The spin-3/2 and spin-5/2 eigenmodes of the Dirac operator with arbitrary imaginary mass parameter on N -dimensional (N ≥ 3) de Sitter spacetime (dS N ) are obtained by analytic continuation. Their transformation properties under the de Sitter algebra spin(N, 1) are studied. For N odd, we show that there is no de Sitter (dS) invariant scalar product for these eigenmodes. For N even, although dS invariant scalar products exist, positive-definiteness of the norm occurs only for the strictly and partially massless theories in N = 4 dimensions. For N = 4, the way in which the eigenmodes form unitary strictly and partially massless representations of spin(4, 1) is emphasised. The analysis presented in this paper reveals previously unknown features of the gauge-invariant theories with spin 3/2 and 5/2 on dS N (N ≥ 3): the strictly massless spin-3/2 field theory, as well as the strictly and partially massless spin-5/2 field theories, are unitary only for N = 4. In particular, a unitary theory for the gravitino field on dS N does not exist unless N = 4.