“…Fortunately, an original ε-polytype structure of GaSe is strengthening by isovalent element doping as well other physical properties responsible for frequency conversion efficiency are modifying that, respectively, allowed easier cut & polishing at arbitrary directions and improves in the frequency conversion efficiency. Strengthened structure gives opportunity of the application in out-of-door applied systems 10 . Modified properties and improved efficiencies are reported for a number of doped crystals: light (GaSe:S) and heavely S-doped GaSe crystals or so called solid solution crystals GaSe 1-x S x (GaSe:GaS) 11,12,13,14,15 , GaSe:In and Ga 1-x In x Se 16,17,18,19,20 , GaSe:Te and GaSe 1-x Te x 18,21,22 , doped GaSe:Er 23,24 and GaSe:Al 25 crystals.…”