2019
DOI: 10.1016/j.ijheatmasstransfer.2019.02.015
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The effects of exothermic catalytic reactions upon combined transport of heat and mass in porous microreactors

Abstract: Microreactors for chemical synthesis and combustion have already attracted significant attention. Exothermic catalytic activity features heavily in these devices and thus advective-diffusive transport is of key importance in their analyses. Yet, thermal modelling of the heat generated by catalytic reactions on the internal surfaces of porous microreactors has remained as an important unresolved issue. To address this, the diffusion of heat of catalytic reactions into three phases including fluid, porous solid … Show more

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Cited by 58 publications
(17 citation statements)
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“…The volumetric rate of local entropy generation in the porous region of the problem can be expressed by the following relation [44][45][46][47][48]:…”
Section: Entropy Generationmentioning
confidence: 99%
“…The volumetric rate of local entropy generation in the porous region of the problem can be expressed by the following relation [44][45][46][47][48]:…”
Section: Entropy Generationmentioning
confidence: 99%
“…The problem outlined in Section "Theoretical and numerical methods" was solved using various non-dimensional and dimensional parameters that are presented for quantitative analysis by the default values in Tables 2 and 3, respectively. It is noted that the values of parameters in Table 2 were chosen in a way that the results become comparable with the existing data in the literature for Newtonian fluids [1,3].…”
Section: Description Of the System Configurationmentioning
confidence: 71%
“…Catalytic porous microchannels, where catalytic channels of small sizes filled with porous media, have received increased interest in traditional and advanced chemical and energy technologies in the last decade. Featuring high surface-tovolume ratios, catalytic porous microchannels can readily achieve the desired performance on transport and chemical reactions [1][2][3]. Therefore, extensive studies have been reported in recent years on applications of catalytic porous microchannels [4][5][6][7].…”
Section: Introductionmentioning
confidence: 99%
“…Considering a strongly temperature-dependent reaction rate and thermal diffusion of mass (Soret effects), the conservation of chemical species becomes [39,41,42]…”
Section: The Studied Configuration Governing Equations and Assumptionsmentioning
confidence: 99%