a b s t r a c tWe report results from monitoring Pluto's 0.8 to 2.4 lm reflectance spectrum with IRTF/SpeX on 65 nights over the dozen years from 2001 to 2012. The spectra show vibrational absorption features of simple molecules CH 4 , CO, and N 2 condensed as ices on Pluto's surface. These absorptions are modulated by the planet's 6.39 day rotation period, enabling us to constrain the longitudinal distributions of the three ices. Absorptions of CO and N 2 are concentrated on Pluto's anti-Charon hemisphere, unlike absorptions of less volatile CH 4 ice that are offset by roughly 90°from the longitude of maximum CO and N 2 absorption. In addition to the diurnal variations, the spectra show longer term trends. On decadal timescales, Pluto's stronger CH 4 absorption bands have been getting deeper, while the amplitude of their diurnal variation is diminishing, consistent with additional CH 4 absorption at high northern latitudes rotating into view as the sub-Earth latitude moves north (as defined by the system's angular momentum vector). Unlike the CH 4 absorptions, Pluto's CO and N 2 absorptions appear to be declining over time, suggesting more equatorial or southerly distributions of those species. Comparisons of geometrically-matched pairs of observations favor geometric explanations for the observed secular changes in CO and N 2 absorption, although seasonal volatile transport could be at least partly responsible. The case for a volatile transport contribution to the secular evolution looks strongest for CH 4 ice, despite it being the least volatile of the three ices.