2024
DOI: 10.1002/adfm.202404434
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The Key Role of Grain Boundary Dynamics in Revolutionizing the Potential of Solid Electrolytes

Yangyang Wang,
Charlotte Thomas,
Kaitlin Garman
et al.

Abstract: Solid electrolytes (SEs) have the potential to enhance the safety and performance of Li‐metal batteries. However, the existence of grain boundaries in polycrystalline SEs presents a significant challenge for both ionic and electronic migration, promoting the propagation of detrimental lithium dendrites. This study compares the roles of grain boundaries in electrical properties of three distinct SEs including garnet‐type Li6.5La3Zr1.5Ta0.5O12 (LLZO), argyrodite‐type Li6PS5Cl (LPSC), and NASICON‐type Li1+x+yAlx(… Show more

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