The phenomenon of “dead” metal in heterogeneous catalysis: opportunities for increasing the efficiency of carbon-supported metal catalysts

Mironenko, Roman M.; Eremin, Dmitry B.; Ananikov, Valentine P.

doi:10.1039/d3sc04691e

Chem. Sci.

2023

DOI: 10.1039/d3sc04691e

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The phenomenon of “dead” metal in heterogeneous catalysis: opportunities for increasing the efficiency of carbon-supported metal catalysts

Roman M. Mironenko,

Dmitry B. Eremin,

Valentine P. Ananikov

Abstract: The key factors contributing to the formation of “dead” metal – the fraction of metal in supported catalysts that remains inaccessible to reactants – are examined. Strategies to minimize the formation of “dead” metal are analyzed.

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2024

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Cited by 5 publications

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Effect of the Surface Functionality of Nanoglobular Carbon Altered by its Thermal Treatment on the Formation and Performance of the Pd/NGC Hydrogenation Catalyst

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The phenomenon of “dead” metal in heterogeneous catalysis: opportunities for increasing the efficiency of carbon-supported metal catalysts

Abstract: The key factors contributing to the formation of “dead” metal – the fraction of metal in supported catalysts that remains inaccessible to reactants – are examined. Strategies to minimize the formation of “dead” metal are analyzed.

Cited by 5 publications

References 77 publications

Effect of the Surface Functionality of Nanoglobular Carbon Altered by its Thermal Treatment on the Formation and Performance of the Pd/NGC Hydrogenation Catalyst

Effect of the Surface Functionality of Nanoglobular Carbon Altered by its Thermal Treatment on the Formation and Performance of the Pd/NGC Hydrogenation Catalyst

Analysis of the intermediates of the catalytic system for the Chan—Evans—Lam reaction based on Cu(i) complex with N-heterocyclic carbene

Reactivity and Mechanism of Recoverable Pd₁@C₃N₄ Single-Atom Catalyst in Buchwald–Hartwig Aminations

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The phenomenon of “dead” metal in heterogeneous catalysis: opportunities for increasing the efficiency of carbon-supported metal catalysts

Abstract: The key factors contributing to the formation of “dead” metal – the fraction of metal in supported catalysts that remains inaccessible to reactants – are examined. Strategies to minimize the formation of “dead” metal are analyzed.

Cited by 5 publications

References 77 publications

Effect of the Surface Functionality of Nanoglobular Carbon Altered by its Thermal Treatment on the Formation and Performance of the Pd/NGC Hydrogenation Catalyst

Effect of the Surface Functionality of Nanoglobular Carbon Altered by its Thermal Treatment on the Formation and Performance of the Pd/NGC Hydrogenation Catalyst

Analysis of the intermediates of the catalytic system for the Chan—Evans—Lam reaction based on Cu(i) complex with N-heterocyclic carbene

Reactivity and Mechanism of Recoverable Pd1@C3N4 Single-Atom Catalyst in Buchwald–Hartwig Aminations

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Reactivity and Mechanism of Recoverable Pd₁@C₃N₄ Single-Atom Catalyst in Buchwald–Hartwig Aminations