The photocatalytic ability of visible-light-responsive interfacial charge transfer complex between TiO2 and Tiron

Lazić, Vesna; Sredojević, Dušan; Ćirić, Aleksandar; Nedeljković, Jovan M.; Zelenková, Gabriela; Férová, Marta; Zelenka, Tomáš; Chavhan, Madhav Prabhakar; Slovák, Václav

doi:10.1016/j.jphotochem.2023.115394

Journal of Photochemistry and Photobiology A: Chemistry

2024

DOI: 10.1016/j.jphotochem.2023.115394

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The photocatalytic ability of visible-light-responsive interfacial charge transfer complex between TiO2 and Tiron

Vesna Lazić,

Dušan Sredojević,

Aleksandar Ćirić

et al.

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2024

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Cited by 2 publications

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Photoinduced reactive species in interfacial charge transfer complex between TiO2 and taxifolin: DFT and EPR study

Nikšić,

Malček Šimunková,

Dyrčíková

et al. 2024

Optical Materials

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Photoinduced reactive species in interfacial charge transfer complex between TiO2 and taxifolin: DFT and EPR study

Nikšić,

Malček Šimunková,

Dyrčíková

et al. 2024

Optical Materials

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Photocatalytic Reactions over TiO2-Based Interfacial Charge Transfer Complexes

Lazić,

Nedeljković

2024

Catalysts

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The present review is related to the novel approach for improvement of the optical properties of wide bandgap metal oxides, in particular TiO2, based on the formation of the inorganic–organic hybrids that display absorption in the visible spectral range due to the formation of interfacial charge transfer (ICT) complexes. We outlined the property requirements of TiO2-based ICT complexes for efficient photo-induced catalytic reactions, emphasizing the simplicity of the synthetic procedure, the possibility of the fine-tuning of the optical properties supported by the density functional theory (DFT) calculations, and the formation of a covalent linkage between the inorganic and organic components of hybrids, i.e., the nature of the interface. In addition, this study provides a comprehensive insight into the potential applications of TiO2-based ICT complexes in photo-driven catalytic reactions (water splitting and degradation of organic molecules), including the identification of the reactive species that participate in photocatalytic reactions by the spin-trapping electron paramagnetic resonance (EPR) technique. Considering the practically limitless number of combinations between the inorganic and organic components capable of forming oxide-based ICT complexes and with the knowledge that this research area is unexplored, we are confident it is worth studying, and we emphasized some further perspectives.

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The photocatalytic ability of visible-light-responsive interfacial charge transfer complex between TiO2 and Tiron

Cited by 2 publications

References 51 publications

Photoinduced reactive species in interfacial charge transfer complex between TiO2 and taxifolin: DFT and EPR study

Photoinduced reactive species in interfacial charge transfer complex between TiO2 and taxifolin: DFT and EPR study

Photocatalytic Reactions over TiO2-Based Interfacial Charge Transfer Complexes

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