This is a report of multi-parameter mineral magnetic results of the Sanmenxia loess-paleosol couplets in the SE extremity of the Chinese Loess Plateau (CLP) over the interval of L1-L13 spanning the last 1 Ma. These results show that mass-specific magnetic susceptibility (χ), χ ARM and SIRM and their ratios exhibit parallel stratigraphic variations. Since superparamagnetic (SP) particles have significant contribution to χ but no contribution to remanence, e.g., ARM and SIRM, the strong linear correlations between χ and remanence (e.g., ARM and SIRM) suggest that the pedogenesis-produced magnetic grains are predominantly in small single domain range. Consequently, the significant contribution of SP particles to the bulk χ as supposed in previous studies has been obviously overestimated.χ ARM /χ data in Sanmenxia and median grain size records of typical loess sections from the hinterland of the CLP display a strong resemblance, implying that χ ARM /χ may be regarded as a reliable indicator for monitoring the variations of ferrimagnetic grain sizes. The results of S-ratio and HIRM ((SIRM+IRM −0.3T )/2) measurements indicate that there is significant enhancement of both soft magnetite/maghemite and hard hematite/goethite in paleosols associated with pedogenesis.Presently it is widely accepted that the enhancement of magnetic susceptibility for the Chinese loess-paleosol sequences is primarily due to the formation of ultrafine magnetic particles through pedogenesis [1] . However, there still exist controversies on both the actual contribution of pedogenesis-produced superparamagnetic (SP) particles to the total magnetic susceptibility and the process whereby climate change is encoded in magnetic susceptibility signals [ ] 2-5 . Relying on a specific multiple regression technique to fit the experimental isothermal and anhysteretic remanent magnetization data to corresponding data for synthetic analogues, Maher and Thompson [6] demonstrate that the contribution of magnetite in soils is twice as much as in loess, and over 90% of the susceptibility contrast between soil and loess is due to magnetic grains lying near the SP threshold. Based on low-temperature saturation remanence magnetization analysis, Banerjee and Hunt [7] suggest that the ratios of SP/total saturation remanence at 15 K are as high as about 0.75 in soil but only 0.2 in loess. Results of detailed magnetic susceptibility measurements and grain size analysis by Han and Jiang [8] suggest that the very fine-grained particles (<0.3 μm), which are considered to be of pedogenic origin, contribute little to the bulk magnetic susceptibility, no more than 3%. Recently, Liu et al. [9 11] report thorough enquiries into the grain-size distribution, concentration and enhancement mechanisms of magnetic minerals in Chinese loess by a series of fruitful rock magnetic measurements. These detailed mineral magnetic results from the western Chinese Loess Plateau (CLP) suggest that: 1) single-domain (SD) magnetic particles contribute more than half of the magnetic susceptibi...