The synthesis of MOF derived carbon and its application in water treatment

Ding, Jiani; Tang, Yijian; Zheng, Shasha; Zhang, Songtao; Xue, Huaiguo; Kong, Qingquan; Pang, Huan

doi:10.1007/s12274-022-4327-1

Cited by 57 publications

(22 citation statements)

References 235 publications

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“…9 Recently, MOF-derived carbons (MDCs), a class of derived carbon materials obtained through the pyrolysis of metalorganic frameworks (MOFs), have attracted a great deal of attention from researchers. 10,11 Most MOFs are less stable and tend to self-decompose in the aqueous phase, limiting their use in the removal of environmental pollutants. Unlike MOFs, MDCs have good thermal/chemical stability, variable surface chemistry and ease of surface modication, making them superior for the adsorption of a wide range of pollutants in water.…”

Section: Introductionmentioning

confidence: 99%

“…Unlike MOFs, MDCs have good thermal/chemical stability, variable surface chemistry and ease of surface modication, making them superior for the adsorption of a wide range of pollutants in water. [10][11][12] However, due to the limited active functional groups on pure MDC, its adsorption performance needs to be further improved. In order to improve the adsorption capacity of carbon-based adsorbents, it is important to introduce sufficient functional groups on the surface of the carbon material for the target material.…”

Section: Introductionmentioning

confidence: 99%

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Amine-functionalized MOF-derived carbon materials for efficient removal of Congo red dye from aqueous solutions: simulation and adsorption studies

Hou

et al. 2023

RSC Adv.

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Section: Introductionmentioning

confidence: 99%

Section: Introductionmentioning

confidence: 99%

Amine-functionalized MOF-derived carbon materials for efficient removal of Congo red dye from aqueous solutions: simulation and adsorption studies

Hou

et al. 2023

RSC Adv.

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“…Subsequent pyrolysis gives rise to an amorphous or graphitic carbon coating on the metal compounds [ 24 ]. Up until now, the usage of metal–organic frameworks (MOFs) as the parent precursor to access metal-containing carbon materials has been variously reported [ 25 , 26 , 27 , 28 ]. Compared with the conventional one, the MOF-derived route can retain the morphology and structure of the parent MOF, allowing facile regulation of the resulting compositions and structures, especially the porosity [ 29 ].…”

Section: Introductionmentioning

confidence: 99%

Coronavirus-Like Core–Shell-Structured Co@C for Hydrogen Evolution via Hydrolysis of Sodium Borohydride

Chen

Yang

et al. 2023

Molecules

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Constructing a reliable and robust cobalt-based catalyst for hydrogen evolution via hydrolysis of sodium borohydride is appealing but challenging due to the deactivation caused by the metal leaching and re-oxidization of metallic cobalt. A unique core–shell-structured coronavirus-like Co@C microsphere was prepared via pyrolysis of Co-MOF. This special Co@C had a microporous carbon coating to retain the reduced state of cobalt and resist the metal leaching. Furthermore, several nano-bumps grown discretely on the surface afforded enriched active centers. Applied in the pyrolysis of NaBH4, the Co@C-650, carbonized at 650 °C, exhibited the best activity and reliable recyclability. This comparable performance is ascribed to the increased metallic active sites and robust stability.

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“…3,4 Carbon materials with sp, sp 2 , and sp 3 hybrid state have a variety of allotropes, which have been widely used in fundamental research. [5][6][7] Among these allotropes, GDY has a two-dimensional structure composed of sp 2 -hybridized benzene rings and sp-hybridized butadiyne linkers. 8,9 Since GDY was first successfully prepared via the Glaser-Hay reaction on a copper substrate, 10 the design and preparation of GDY can give rise to widespread research enthusiasm.…”

Section: Introductionmentioning

confidence: 99%

Fabrication of graphdiyne and its analogues for photocatalytic application

Liang

Deng

Zhou

et al. 2022

EcoMat

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Graphdiyne (GDY), an emerging two‐dimensional all‐carbon allotrope, features the coexistence of sp and sp2 hybridized planar carbon atoms. GDY and GDY‐based materials exhibit unique physical and chemical properties, such as well‐defined molecular skeleton, π‐conjugated structure, high specific surface area with porosity, and good electrical conductivity, which have aroused widespread interest in various disciplines. As an emerging field, in this work, we summarize important synthesis strategies of GDY and GDY‐based materials including classical synthesis, chemical vapor deposition, explosion approach, and interface‐assisted methods. We also elaborate the recent modifications to regulate the structure and properties of GDY from the viewpoint of metal doping, non‐metal doping, and heterostructure construction. Meanwhile, recent achievements and progress in the development of energy and environmental applications in photocatalysis are highlighted. Lastly, the challenges and potential developments of GDY in the catalytic research are given at the end of this article.

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The synthesis of MOF derived carbon and its application in water treatment

Cited by 57 publications

References 235 publications

Amine-functionalized MOF-derived carbon materials for efficient removal of Congo red dye from aqueous solutions: simulation and adsorption studies

Amine-functionalized MOF-derived carbon materials for efficient removal of Congo red dye from aqueous solutions: simulation and adsorption studies

Coronavirus-Like Core–Shell-Structured Co@C for Hydrogen Evolution via Hydrolysis of Sodium Borohydride

Fabrication of graphdiyne and its analogues for photocatalytic application

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