Geochemical studies of sandstones from the three lithostratigraphic successions in the southern Benue Trough of Nigeria were undertaken for a geochemical characterization of the sandstones, and to assess their stratigraphic and source evolution.Major and trace elements data were obtained from outcrop sandstone samples. The SiO 2 /Al 2 O 3 , Fe 2 O 3 /K 2 O ratios and CaO contents have been used to characterize the Cretaceous sandstones into Al-rich and high and low Fe 2 O 3 /K 2 O ratio sandstones. Results indicate that there are geochemical features that display stratigraphic trends across the succession from the Asu River Group, Eze-Aku Group to the proto-Niger Delta succession which may imply a discontinuous evolution from different source terrains of Precambrian and Mesozoic ages that supplied the sediments. The Asu River Group sandstones have lower SiO 2 , Al 2 O 3 , Fe 2 O 3 and higher MgO; the Eze-Aku sandstones have higher TiO 2 , CaO, alkalis and lower MgO while the proto-Niger Delta sandstones have higher SiO 2 , Al 2 O 3 , Fe 2 O 3 and lower alkalis and CaO. These discontinuities signify the influence of tectonic impulses that affected the southern Benue Trough during the Cretaceous time. Changes in ratios of TiO 2 /Al 2 O 3 , Fe 2 O 3 , Cr and Zr suggest an increasingly mafic contribution to the depositional basin with time. The chemical index of alteration increases with time, possibly suggesting that a more intense weathering regime in the hinterland developed with time.