2023
DOI: 10.1002/hlca.202300079
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The π‐Molecular Complex of Biphenylene and Tetracyanoethylene

Rita Dobszay,
Péter J. Mayer,
Tamás Holczbauer
et al.

Abstract: The investigation of the biphenylene (BP)‐tetracyanoethylene (TCNE) π‐molecular complex is reported. The first study on this complex appeared in 1961 and was considered as a charge transfer complex with a symmetric, co‐planar arrangement of the components. Moreover, it was assumed that this arrangement is not only dictated by the formation of a Mulliken‐type donor‐acceptor complex, but also by the electronic stabilization of the “cyclobutadieneoid” central ring of biphenylene through complex formation. Yet, cr… Show more

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