Theoretical investigation of photoprocesses in complex organic compounds upon high-power laser excitation

Abstract

A procedure of theoretical investigations into the dynamics of energy level populations of organic molecules upon high-power laser excitation is developed that allows information on stimulated emission of molecules, gain and lasing spectra, dynamics of lasing pulses, populations of the ground and excited states, and influence of the induced absorption on lasing of the organic molecules to be obtained. Laws of changing of the aboveindicated processes are established for two pyran substitutes. Results of theoretical and experimental investigations are well correlated.