Theoretical prediction of a carrier gas effect under nucleation in thermal diffusion chambers

Itkin, A. L.

doi:10.1016/s0301-0104(00)00067-7

Chemical Physics

2000

DOI: 10.1016/s0301-0104(00)00067-7

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Theoretical prediction of a carrier gas effect under nucleation in thermal diffusion chambers

A. L. Itkin¹

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2001

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The Impact of Convective Flow on Thermal Diffusion Cloud Chamber Operation

Heist

Ferguson

2001

J. Phys. Chem. B

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We report here new results that further elucidate the role of buoyancy-driven convective flows in determining the distribution of vapor mole fraction and temperature in the thermal diffusion cloud chamber. A two-dimensional model describing both diffusion and convection in the presence of chamber sidewalls is presented. The model equations are used to analyze 1-butanol and 1-pentanol nucleation data obtained earlier. The results of the investigation show that convective flow is nearly always present and, in the cases considered here, result in a reduction in the value of the calculated critical supersaturation (as compared to the one-dimensional case). The dependence of critical supersaturation with total pressure reported earlier is smaller but is not eliminated.

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The Impact of Convective Flow on Thermal Diffusion Cloud Chamber Operation

Heist

Ferguson

2001

J. Phys. Chem. B

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Kinetic Model of Effect of a Carrier Gas on Nucleation in a Diffusion Chamber

Itkin¹

2001

Aerosol Science and Technology

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Theoretical prediction of a carrier gas effect under nucleation in thermal diffusion chambers

Cited by 2 publications

References 20 publications

The Impact of Convective Flow on Thermal Diffusion Cloud Chamber Operation

The Impact of Convective Flow on Thermal Diffusion Cloud Chamber Operation

Kinetic Model of Effect of a Carrier Gas on Nucleation in a Diffusion Chamber

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