We have measured surface morphology and gas adsorption characteristics of uncompressed pyrolytic graphite sheet (uPGS) which is a candidate substrate for AC and DC superflow experiments on monolayers of 4 He below T = 1 K. The PGS is a mass-produced thin graphite sheet with various thicknesses between 10 and 100 µm. We employed a variety of measuring techniques such as imagings with optical microscope, SEM and STM, Raman spectroscopy, and adsorption isotherm. PGS has smooth and atomically-flat external surfaces with high crystallinity. Although the specific surface area (≤ 0.1 m 2 /g) is rather small, by making use of its smooth external surface, the thinnest uPGS of 10 µm thick is found to be suitable for the superflow experiments on the strictly two-dimensional helium systems.A few atomic layers of helium (He) adsorbed on graphite substrate are experimental realization of correlated two-dimensional (2D) quantum systems. New types of superfluidity, which should not be a simple extrapolation of thin superfluid 4 He films of several tens atomic layers thick, are expected there. Crowell and Reppy [1] found a novel superfluidity below 400 mK, which is reentrant as