2022
DOI: 10.1021/acs.jpca.2c04530
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Thermionic Emission of Negative Ions of Molecules and Small Clusters as a Probe of Low-Energy Attachment

Abstract: We have been studying the thermionic emission of negatively charged molecules and small clusters for more than a decade. The kinetic energy released distribution (KERD) of mass-selected negative ions has been measured with a velocity map imaging spectrometer. A comparison of the experimental KERD to detailed balance models provided information on the reverse process, namely, the electron attachment to the parent. The electron attachment to neutral systems (reverse process of the electron emission from anions) … Show more

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