2000
DOI: 10.1006/jcht.1999.0564
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Thermodynamic study of the Na-Cu-Cl-SO - H O system at the temperature 298.15 K

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Cited by 30 publications
(45 citation statements)
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References 23 publications
(50 reference statements)
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“…The simulation is based on the following procedure: determination of the Pitzer binary parameters β (0) , β (1) , and C φ taking into account the ionic interactions of two ions and three ions; determination of the Pitzer ternary parameters {θ(MN) and (MNX)} characterizing the interaction between two different ions of the same sign (MN) and the interaction between three ions (MNX, MMX and NNX), respectively; and calculation of the solubility isotherms of the three-component solutions. The same scheme has been used to simulate other ternary (5,7,(15)(16)(17) and multicomponent solutions (18,19) from which phases with a constant stoichiometric composition (simple or double salts) crystallize. The parameters of ionic interaction of the binary subsystems have been determined by many authors.…”
Section: Calculation Of Solubilitymentioning
confidence: 99%
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“…The simulation is based on the following procedure: determination of the Pitzer binary parameters β (0) , β (1) , and C φ taking into account the ionic interactions of two ions and three ions; determination of the Pitzer ternary parameters {θ(MN) and (MNX)} characterizing the interaction between two different ions of the same sign (MN) and the interaction between three ions (MNX, MMX and NNX), respectively; and calculation of the solubility isotherms of the three-component solutions. The same scheme has been used to simulate other ternary (5,7,(15)(16)(17) and multicomponent solutions (18,19) from which phases with a constant stoichiometric composition (simple or double salts) crystallize. The parameters of ionic interaction of the binary subsystems have been determined by many authors.…”
Section: Calculation Of Solubilitymentioning
confidence: 99%
“…Using the foregoing model The solubility isotherms of the ternary solutions at T = 298.15 K are calculated on the basis of the thermodynamic functions obtained. A method described in previous papers (15)(16)(17)(18)(19) has been used. At phase and chemical equilibrium of a given salt (l 1 A 1 · l 2 A 2 · l 3 A 3 ) with its saturated solution, the following equation applies:…”
Section: Calculation Of Solubilitymentioning
confidence: 99%
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“…(15) It has been shown that Pitzer equations can describe the properties of binary (1,2,4,13) and multicomponent (16,17) solutions in which phases with a constant composition (simple and double salts) (16)(17)(18)(19)(20) and solid solutions (3,5) crystallize.…”
Section: Calculation Of the Solubilitymentioning
confidence: 99%
“…The applicability of this approach has been shown for a series of other ternary and multicomponent aqueous solutions. (16)(17)(18)(19)(20) BINARY SUBSYSTEMS A thermodynamic analysis of Cs 2 SeO 4 (aq) has been performed on the basis of the data obtained in the present study on the concentration dependence of the osmotic coefficient (table 1). The binary parameters of the interionic interaction for NiSeO 4 (aq) are taken from the literature.…”
Section: Calculation Of the Solubilitymentioning
confidence: 99%