NdTbCo/Cr amorphous fi lms with high perpendicular magnetic anisotropy were prepared onto glass substrates by rf magnetron sputtering. The effects of Nd substitution on the magnetic and magneto-optical properties of TbCo/Cr fi lms were investigated. It was found that partial Tb substitution by Nd would increase the saturation magnetization and the Kerr rotation angle, change the temperature dependence of magneto-optical characteristics. These results can be explained by the ferrimagnetic structure of the rare earth-transition metal alloy. When the magnetic layer composition was (Nd 0.265 Tb 0.735 ) 31 Co 69 , a saturation magnetization of 247 emu/ cm 3 and a coercivity of 3.8 kOe at room temperature could be obtained.