“…Wearable electronic devices have garnered significant attention for their tremendous potential in enabling intelligent systems, , monitoring human physiological signals, , and contributing to the Internet of Things. , Flexible pressure/force sensors, − as vital components of wearable electronic devices, find wide applications across various fields, including human health monitoring, disease diagnosis, and motion detection. Among the diverse range of flexible pressure sensors, piezoresistive sensors have gained immense interest due to their ease of fabrication, efficient signal collection, stable mechanical–electrical properties, and high sensitivity. , However, despite notable progress in developing flexible piezoresistive sensors, − challenges persist in fabricating sensors with excellent overall performances that can fully meet the demands of wearable electronic devices, particularly regarding high sensitivity over a broad sensing range. − Furthermore, most traditional flexible piezoresistive sensors typically use polymers as substrates, such as poly(dimethylsiloxane) (PDMS), , poly(ethylene terephthalate) (PET), , and polyurethane (PU). , Nevertheless, these substrates are unsuitable for long-term wear, potentially causing skin inflammation and itching due to poor air permeability, thereby limiting their application in human health monitoring. Moreover, these elastic substrates are challenging to degrade, resulting in the rapid accumulation of electronic waste and posing a serious threat to the environment with the widespread use of wearable electronic products.…”