Time-Dependent Unitary Transformation Method in the Strong-Field-Ionization Regime with the Kramers-Henneberger Picture

Abstract

Time evolution operators of a strongly ionizing medium are calculated by a time-dependent unitary transformation (TDUT) method. The TDUT method has been employed in a quantum mechanical system composed of discrete states. This method is especially helpful for solving molecular rotational dynamics in quasi-adiabatic regimes because the strict unitary nature of the propagation operator allows us to set the temporal step size to large; a tight limitation on the temporal step size (δt<<1) can be circumvented by the strict unitary nature. On the other hand, in a strongly ionizing system where the Hamiltonian is not Hermitian, the same approach cannot be directly applied because it is demanding to define a set of field-dressed eigenstates. In this study, the TDUT method was applied to the ionizing regime using the Kramers-Henneberger frame, in which the strong-field-dressed discrete eigenstates are given by the field-free discrete eigenstates in a moving frame. Although the present work verifies the method for a one-dimensional atom as a prototype, the method can be applied to three-dimensional atoms, and molecules exposed to strong laser fields.

Laser-Dressed Molecular Point Groups in the Kramers–Henneberger Oscillating Frame-of-Reference: Selection Rules for Higher Harmonic Generation

“…the Kramers–Henneberger representation, , the form of the equation involves a time-dependent space-translation. A recent work by Mun et al uses a time-dependent unitary transformation method to describe strong-field ionization within the Kramers–Henneberger picture. In this work, we use the Kramers–Henneberger (KH) formalism , to define dynamical symmetries.…”