Abstract:We have developed a new instrument for monitoring elec tronic wavepacket dynamics using a single electromagnetic pulse pair. The operation of the device is analogous to that of single-shot cross correlators commonly used to monitor the temporal evolution of short laser pulses. We have used the instrument to probe wavepacket evo lution over time scales ranging from 100 psec to less than 1 fsec. The device reduces the amount of time required to collect pump-probe time delay data by orders of magnitude, greatly reducing the deleterious ef fects of experimental drifts. In addition, the single-shot feature provides real-time feedback as to the affect of various experimental parameters on the electron dynamics, allowing us to literally tune-up our equip ment to enhance desired behavior at specific times.