2023
DOI: 10.1021/acsnano.3c05974
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Topological Design and Synthesis of High-Spin Aza-triangulenes without Jahn–Teller Distortions

James Lawrence,
Yuanyuan He,
Haipeng Wei
et al.

Abstract: The atomic doping of open-shell nanographenes enables precise tuning of their electronic and magnetic states, which is crucial for their promising potential applications in optoelectronics and spintronics. Among this intriguing class of molecules, triangulenes stand out with their size-dependent electronic properties and spin states, which can also be influenced by the presence of dopant atoms and functional groups. However, the occurrence of Jahn–Teller distortions in such systems can have a crucial impact on… Show more

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Cited by 9 publications
(1 citation statement)
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“…Apart from this, it is also of great importance to perform those precise fabrications of open-shell nanographenes and heteroatom-doped nanographenes (e.g., Aza-triangulenes , ) on different surfaces and solid devices, such as graphene-based devices (Figure b) . It has been predicted that the external electric field can be used to switch on and off the π-magnetism of zigzag-edged π-magnets by charging effect .…”
Section: Summary and Perspectivementioning
confidence: 99%
“…Apart from this, it is also of great importance to perform those precise fabrications of open-shell nanographenes and heteroatom-doped nanographenes (e.g., Aza-triangulenes , ) on different surfaces and solid devices, such as graphene-based devices (Figure b) . It has been predicted that the external electric field can be used to switch on and off the π-magnetism of zigzag-edged π-magnets by charging effect .…”
Section: Summary and Perspectivementioning
confidence: 99%