In order to develop a laser-driven spin-polarized 3He-ion beam source available for nuclear-physics experiments as well as for the investigation of polarized nuclear fusion, several challenges have to be overcome. Apart from the provision of a properly polarized 3He gas-jet target, one of the biggest milestones is the demonstration of the general feasibility of laser-induced ion acceleration out of gas-jet targets. Of particular importance is the knowledge about the main ion-emission angles as well as the achievable ion-energy spectra (dependent on the optimal set of laser and target parameters). We report on the results of such a feasibility study performed at PHELIX, GSI Darmstadt. Both 3He- and 4He-gas jets (n
gas ∼ 1019 cm−3) were illuminated with high-intensity laser pulses,
I
L
∼
(
10
19
W
cm
−
2
)
. The main ion-emission angles could be identified (±90° with respect to the laser-propagation direction) and the ion-energy spectra for all ion species could be extracted: for the optimal laser and target parameters, the high-energy cut-offs for He
2
+
,
1
+
ions were 4.65 MeV (with a normalized energy uncertainty of
Δ
−
1
=
0.033
) and 3.27 MeV (
Δ
−
1
=
0.055
), respectively.