Towards maximizing the In2O3/m-ZrO2 interfaces for CO2-to-methanol hydrogenation

Luo, Alin; Chang, Haohao; Gao, Feifan; Liu, Yongmei; He, Heyong; Cao, Yong

doi:10.1039/d3cc04260j

Chem. Commun.

2023

DOI: 10.1039/d3cc04260j

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Towards maximizing the In₂O₃/m-ZrO₂ interfaces for CO₂-to-methanol hydrogenation

Alin Luo,

Haohao Chang,

Feifan Gao

et al.

Abstract: The incorporation of diethylenetriaminepenta-acetic acid (DTPA) as a chelating agent resulted in abundant Zr–O–In structures at the catalyst interface, leading to exceptional CO2-to-methanol activity.

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2024

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Comprehensive Insight into Indium Oxide‐Based Catalysts for CO₂ Hydrogenation: Thermal, Photo, and Photothermal Catalysis

Shi,

Yang,

et al. 2024

Adv Funct Materials

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The conversion of carbon dioxide (CO2) into value‐added chemicals presents an innovative pathway for advancing the low‐carbon clean energy revolution, contributing significantly to CO2 emission reduction and resource utilization. Recently, In2O3‐based catalysts have emerged as a promising frontier in CO2 hydrogenation research. This review provides a comprehensive introduction of the latest advancements in the application of In2O3‐based catalysts across thermal, photocatalytic, and photothermal catalysis platforms. The review examines critical aspects such as structural properties, active sites, reaction mechanisms, performance enhancement, product impact, and the development of multi‐functional catalytic systems. Thermal Catalysis for CO2 hydrogenation involves the application of elevated temperatures to initiate and drive the hydrogenation reactions. Photocatalysis, on the other hand, harnesses light energy to facilitate these reactions. Among these approaches, photothermal catalysis has emerged as a particularly promising method for CO2 hydrogenation, offering several advantages over both thermal catalysis and photocatalysis. These advantages include more efficient energy utilization, a broader range of reaction conditions, enhanced synergistic effects, selective activation, and improved environmental sustainability. This review not only summarizes the current state of research in this field but also may provide critical insights and guidance for future studies aimed at advancing artificial carbon cycling processes.

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Comprehensive Insight into Indium Oxide‐Based Catalysts for CO₂ Hydrogenation: Thermal, Photo, and Photothermal Catalysis

Shi,

Yang,

et al. 2024

Adv Funct Materials

View full text Add to dashboard Cite

show abstract

In situ DRIFTS and DFT study of CO₂ hydrogenation over the In₂O₃ catalyst

Zou,

Liu,

Shen

et al. 2024

Chem. Commun.

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Boosting CO₂ chemical fixation over MOF-808 by the introduction of functional groups and defective Zr sites

Zhou,

Qu,

Zhang

et al. 2024

Chem. Commun.

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Towards maximizing the In₂O₃/m-ZrO₂ interfaces for CO₂-to-methanol hydrogenation

Abstract: The incorporation of diethylenetriaminepenta-acetic acid (DTPA) as a chelating agent resulted in abundant Zr–O–In structures at the catalyst interface, leading to exceptional CO2-to-methanol activity.

Cited by 3 publications

References 32 publications

Comprehensive Insight into Indium Oxide‐Based Catalysts for CO₂ Hydrogenation: Thermal, Photo, and Photothermal Catalysis

Comprehensive Insight into Indium Oxide‐Based Catalysts for CO₂ Hydrogenation: Thermal, Photo, and Photothermal Catalysis

In situ DRIFTS and DFT study of CO₂ hydrogenation over the In₂O₃ catalyst

Boosting CO₂ chemical fixation over MOF-808 by the introduction of functional groups and defective Zr sites

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Towards maximizing the In2O3/m-ZrO2 interfaces for CO2-to-methanol hydrogenation

Abstract: The incorporation of diethylenetriaminepenta-acetic acid (DTPA) as a chelating agent resulted in abundant Zr–O–In structures at the catalyst interface, leading to exceptional CO2-to-methanol activity.

Cited by 3 publications

References 32 publications

Comprehensive Insight into Indium Oxide‐Based Catalysts for CO2 Hydrogenation: Thermal, Photo, and Photothermal Catalysis

Comprehensive Insight into Indium Oxide‐Based Catalysts for CO2 Hydrogenation: Thermal, Photo, and Photothermal Catalysis

In situ DRIFTS and DFT study of CO2 hydrogenation over the In2O3 catalyst

Boosting CO2 chemical fixation over MOF-808 by the introduction of functional groups and defective Zr sites

Contact Info

Product

Resources

About

Towards maximizing the In₂O₃/m-ZrO₂ interfaces for CO₂-to-methanol hydrogenation

Comprehensive Insight into Indium Oxide‐Based Catalysts for CO₂ Hydrogenation: Thermal, Photo, and Photothermal Catalysis

Comprehensive Insight into Indium Oxide‐Based Catalysts for CO₂ Hydrogenation: Thermal, Photo, and Photothermal Catalysis

In situ DRIFTS and DFT study of CO₂ hydrogenation over the In₂O₃ catalyst

Boosting CO₂ chemical fixation over MOF-808 by the introduction of functional groups and defective Zr sites